Metrological-grade tunable coherent source in the mid-infrared for molecular precision spectroscopy

G. Insero; C. Clivati; D. D'Ambrosio; P. Cancio Pastor; M. Verde; P. G. Schunemann; J. J. Zondy; M. Inguscio; D. Calonico; F. Levi; P. De Natale; G. Santambrogio; S. Borri

doi:10.1117/12.2294025

Metrological-grade tunable coherent source in the mid-infrared for molecular precision spectroscopy

G. Insero, C. Clivati, D. D'Ambrosio, P. Cancio Pastor, M. Verde, P. G. Schunemann, J. J. Zondy, M. Inguscio, D. Calonico, F. Levi, P. De Natale, G. Santambrogio, S. Borri

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

Abstract

We report on a metrological-grade mid-IR source with a 10^-14 short-Term instability for high-precision spectroscopy. Our source is based on the combination of a quantum cascade laser and a coherent radiation obtained by difference-frequency generation in an orientation-patterned gallium phosphide (OP-GaP) crystal. The pump and signal lasers are locked to an optical frequency comb referenced to the primary frequency standard via an optical fiber link. We demonstrate the robustness of the apparatus by measuring a vibrational transition around 6 μm on a metastable state of CO molecuels with 11 digits of precision.

Original language	English
Title of host publication	Nonlinear Frequency Generation and Conversion
Subtitle of host publication	Materials and Devices XVII
Editors	Konstantin L. Vodopyanov, Kenneth L. Schepler
Publisher	SPIE
Volume	10516
ISBN (Electronic)	9781510615175
DOIs	https://doi.org/10.1117/12.2294025
Publication status	Published - Jan 1 2018
Event	Nonlinear Frequency Generation and Conversion: Materials and Devices XVII 2018 - San Francisco, United States Duration: Jan 29 2018 → Jan 31 2018

Publication series

Name	Proceedings of SPIE - The International Society for Optical Engineering
Volume	10516
ISSN (Print)	0277-786X
ISSN (Electronic)	1996-756X

Conference

Conference	Nonlinear Frequency Generation and Conversion: Materials and Devices XVII 2018
Country	United States
City	San Francisco
Period	1/29/18 → 1/31/18

Keywords

Difference frequency generation
Frequency metrology
High-resolution spectroscopy
Laser stabilization
Nonlinear Crystals

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Condensed Matter Physics
Computer Science Applications
Applied Mathematics
Electrical and Electronic Engineering

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Insero, G., Clivati, C., D'Ambrosio, D., Cancio Pastor, P., Verde, M., Schunemann, P. G., Zondy, J. J., Inguscio, M., Calonico, D., Levi, F., De Natale, P., Santambrogio, G., & Borri, S. (2018). Metrological-grade tunable coherent source in the mid-infrared for molecular precision spectroscopy. In K. L. Vodopyanov, & K. L. Schepler (Eds.), Nonlinear Frequency Generation and Conversion: Materials and Devices XVII (Vol. 10516). [105160O] (Proceedings of SPIE - The International Society for Optical Engineering; Vol. 10516). SPIE. https://doi.org/10.1117/12.2294025

Metrological-grade tunable coherent source in the mid-infrared for molecular precision spectroscopy. / Insero, G.; Clivati, C.; D'Ambrosio, D.; Cancio Pastor, P.; Verde, M.; Schunemann, P. G.; Zondy, J. J.; Inguscio, M.; Calonico, D.; Levi, F.; De Natale, P.; Santambrogio, G.; Borri, S.

Nonlinear Frequency Generation and Conversion: Materials and Devices XVII. ed. / Konstantin L. Vodopyanov; Kenneth L. Schepler. Vol. 10516 SPIE, 2018. 105160O (Proceedings of SPIE - The International Society for Optical Engineering; Vol. 10516).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

Insero, G, Clivati, C, D'Ambrosio, D, Cancio Pastor, P, Verde, M, Schunemann, PG, Zondy, JJ, Inguscio, M, Calonico, D, Levi, F, De Natale, P, Santambrogio, G & Borri, S 2018, Metrological-grade tunable coherent source in the mid-infrared for molecular precision spectroscopy. in KL Vodopyanov & KL Schepler (eds), Nonlinear Frequency Generation and Conversion: Materials and Devices XVII. vol. 10516, 105160O, Proceedings of SPIE - The International Society for Optical Engineering, vol. 10516, SPIE, Nonlinear Frequency Generation and Conversion: Materials and Devices XVII 2018, San Francisco, United States, 1/29/18. https://doi.org/10.1117/12.2294025

Insero G, Clivati C, D'Ambrosio D, Cancio Pastor P, Verde M, Schunemann PG et al. Metrological-grade tunable coherent source in the mid-infrared for molecular precision spectroscopy. In Vodopyanov KL, Schepler KL, editors, Nonlinear Frequency Generation and Conversion: Materials and Devices XVII. Vol. 10516. SPIE. 2018. 105160O. (Proceedings of SPIE - The International Society for Optical Engineering). https://doi.org/10.1117/12.2294025

Insero, G. ; Clivati, C. ; D'Ambrosio, D. ; Cancio Pastor, P. ; Verde, M. ; Schunemann, P. G. ; Zondy, J. J. ; Inguscio, M. ; Calonico, D. ; Levi, F. ; De Natale, P. ; Santambrogio, G. ; Borri, S. / Metrological-grade tunable coherent source in the mid-infrared for molecular precision spectroscopy. Nonlinear Frequency Generation and Conversion: Materials and Devices XVII. editor / Konstantin L. Vodopyanov ; Kenneth L. Schepler. Vol. 10516 SPIE, 2018. (Proceedings of SPIE - The International Society for Optical Engineering).

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abstract = "We report on a metrological-grade mid-IR source with a 10-14 short-Term instability for high-precision spectroscopy. Our source is based on the combination of a quantum cascade laser and a coherent radiation obtained by difference-frequency generation in an orientation-patterned gallium phosphide (OP-GaP) crystal. The pump and signal lasers are locked to an optical frequency comb referenced to the primary frequency standard via an optical fiber link. We demonstrate the robustness of the apparatus by measuring a vibrational transition around 6 μm on a metastable state of CO molecuels with 11 digits of precision.",

keywords = "Difference frequency generation, Frequency metrology, High-resolution spectroscopy, Laser stabilization, Nonlinear Crystals",

author = "G. Insero and C. Clivati and D. D'Ambrosio and {Cancio Pastor}, P. and M. Verde and Schunemann, {P. G.} and Zondy, {J. J.} and M. Inguscio and D. Calonico and F. Levi and {De Natale}, P. and G. Santambrogio and S. Borri",

note = "Funding Information: The authors acknowledge financial support from Extreme Light Infrastructure (ELI) European project, from INFN under the SUPREMO project, from Ente Cassa di Risparmio di Firenze under the COSMO project,[] from EMPIR-15SIB05-OFTEN, which has received funding from the EMPIR programme co-financed by the Participating States and from the European Union{\textquoteright}s Horizon 2020 research and innovation programme. Publisher Copyright: {\textcopyright} 2018 SPIE. Copyright: Copyright 2018 Elsevier B.V., All rights reserved.; Nonlinear Frequency Generation and Conversion: Materials and Devices XVII 2018 ; Conference date: 29-01-2018 Through 31-01-2018",

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AU - Levi, F.

AU - De Natale, P.

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N1 - Funding Information: The authors acknowledge financial support from Extreme Light Infrastructure (ELI) European project, from INFN under the SUPREMO project, from Ente Cassa di Risparmio di Firenze under the COSMO project,[] from EMPIR-15SIB05-OFTEN, which has received funding from the EMPIR programme co-financed by the Participating States and from the European Union’s Horizon 2020 research and innovation programme. Publisher Copyright: © 2018 SPIE. Copyright: Copyright 2018 Elsevier B.V., All rights reserved.

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N2 - We report on a metrological-grade mid-IR source with a 10-14 short-Term instability for high-precision spectroscopy. Our source is based on the combination of a quantum cascade laser and a coherent radiation obtained by difference-frequency generation in an orientation-patterned gallium phosphide (OP-GaP) crystal. The pump and signal lasers are locked to an optical frequency comb referenced to the primary frequency standard via an optical fiber link. We demonstrate the robustness of the apparatus by measuring a vibrational transition around 6 μm on a metastable state of CO molecuels with 11 digits of precision.

AB - We report on a metrological-grade mid-IR source with a 10-14 short-Term instability for high-precision spectroscopy. Our source is based on the combination of a quantum cascade laser and a coherent radiation obtained by difference-frequency generation in an orientation-patterned gallium phosphide (OP-GaP) crystal. The pump and signal lasers are locked to an optical frequency comb referenced to the primary frequency standard via an optical fiber link. We demonstrate the robustness of the apparatus by measuring a vibrational transition around 6 μm on a metastable state of CO molecuels with 11 digits of precision.

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KW - Frequency metrology

KW - High-resolution spectroscopy

KW - Laser stabilization

KW - Nonlinear Crystals

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Metrological-grade tunable coherent source in the mid-infrared for molecular precision spectroscopy

Abstract

Publication series

Conference

Keywords

ASJC Scopus subject areas

Access to Document

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