Abstract
Rare Earth- (RE-) doped BiFeO3 (BFO) thin films were grown on LaAlO3 substrates by using pulsed laser deposition technique. All of BFO films doped with 10% of RE show a single phase of rhombohedral structure. The saturated magnetization in the Ho- and Sm-doped films is much larger than those reported in literature and was observed at a quite low field as of 0.2 T. As for Pr- and Nd-doped BFO films, Fe2+ amount is not dominant; thus, ferromagnetism is not favored. As the RE concentration goes up to 20%, all compounds have drastically gone through a structural transition. The RE-doped BFO films have changed from rhombohedral to either pure orthorhombic phase (for Ho, Sm), or a mixed phase of orthorhombic and tetragonal (for Pr, Nd), or pure tetragonal (for Eu). We observed magnetic properties of RE-doped BFO films have significantly changed. While 20% Ho/Sm-doped BFO films have ferromagnetism degraded in comparison with the 10% doping case, the 20% Pr/Nd-doped BFO thin films, whose structure is a mixed phase, have magnetic ordering improved due to the fact that the Fe2+ amount has become greater. It seems that one can control the magnetic properties of BFO films by using appropriate RE dopants and concentrations.
| Original language | English |
|---|---|
| Article number | 371802 |
| Journal | Advances in Condensed Matter Physics |
| Volume | 2015 |
| DOIs | |
| Publication status | Published - 2015 |
| Externally published | Yes |
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ASJC Scopus subject areas
- Condensed Matter Physics
Cite this
Rare earth-doped BiFeO3 thin films : Relationship between structural and magnetic properties. / Thu Huong, Ngo; Lee, Seunghun; Atabaev, Timur Sh; Kurisu, Makio; Hong, Nguyen Hoa.
In: Advances in Condensed Matter Physics, Vol. 2015, 371802, 2015.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - Rare earth-doped BiFeO3 thin films
T2 - Relationship between structural and magnetic properties
AU - Thu Huong, Ngo
AU - Lee, Seunghun
AU - Atabaev, Timur Sh
AU - Kurisu, Makio
AU - Hong, Nguyen Hoa
PY - 2015
Y1 - 2015
N2 - Rare Earth- (RE-) doped BiFeO3 (BFO) thin films were grown on LaAlO3 substrates by using pulsed laser deposition technique. All of BFO films doped with 10% of RE show a single phase of rhombohedral structure. The saturated magnetization in the Ho- and Sm-doped films is much larger than those reported in literature and was observed at a quite low field as of 0.2 T. As for Pr- and Nd-doped BFO films, Fe2+ amount is not dominant; thus, ferromagnetism is not favored. As the RE concentration goes up to 20%, all compounds have drastically gone through a structural transition. The RE-doped BFO films have changed from rhombohedral to either pure orthorhombic phase (for Ho, Sm), or a mixed phase of orthorhombic and tetragonal (for Pr, Nd), or pure tetragonal (for Eu). We observed magnetic properties of RE-doped BFO films have significantly changed. While 20% Ho/Sm-doped BFO films have ferromagnetism degraded in comparison with the 10% doping case, the 20% Pr/Nd-doped BFO thin films, whose structure is a mixed phase, have magnetic ordering improved due to the fact that the Fe2+ amount has become greater. It seems that one can control the magnetic properties of BFO films by using appropriate RE dopants and concentrations.
AB - Rare Earth- (RE-) doped BiFeO3 (BFO) thin films were grown on LaAlO3 substrates by using pulsed laser deposition technique. All of BFO films doped with 10% of RE show a single phase of rhombohedral structure. The saturated magnetization in the Ho- and Sm-doped films is much larger than those reported in literature and was observed at a quite low field as of 0.2 T. As for Pr- and Nd-doped BFO films, Fe2+ amount is not dominant; thus, ferromagnetism is not favored. As the RE concentration goes up to 20%, all compounds have drastically gone through a structural transition. The RE-doped BFO films have changed from rhombohedral to either pure orthorhombic phase (for Ho, Sm), or a mixed phase of orthorhombic and tetragonal (for Pr, Nd), or pure tetragonal (for Eu). We observed magnetic properties of RE-doped BFO films have significantly changed. While 20% Ho/Sm-doped BFO films have ferromagnetism degraded in comparison with the 10% doping case, the 20% Pr/Nd-doped BFO thin films, whose structure is a mixed phase, have magnetic ordering improved due to the fact that the Fe2+ amount has become greater. It seems that one can control the magnetic properties of BFO films by using appropriate RE dopants and concentrations.
UR - http://www.scopus.com/inward/record.url?scp=84941730114&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=84941730114&partnerID=8YFLogxK
U2 - 10.1155/2015/371802
DO - 10.1155/2015/371802
M3 - Article
AN - SCOPUS:84941730114
VL - 2015
JO - Advances in Condensed Matter Physics
JF - Advances in Condensed Matter Physics
SN - 1687-8108
M1 - 371802
ER -